Please use this identifier to cite or link to this item: http://hdl.handle.net/10316/17935
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dc.contributor.authorCardoso, Ana L.-
dc.contributor.authorKaczor, Agnieszka-
dc.contributor.authorSilva, Artur M.S.-
dc.contributor.authorFausto, Rui-
dc.contributor.authorMelo, Teresa M.V.D. Pinho e-
dc.contributor.authorGonsalves, António M. d'A. Rocha-
dc.date.accessioned2011-12-15T15:53:00Z-
dc.date.available2011-12-15T15:53:00Z-
dc.date.issued2006-09-
dc.identifier.urihttp://hdl.handle.net/10316/17935-
dc.description.abstractThe 1,3-dipolar cycloaddition of dimethyl acetylenedicarboxylate with nonstabilized azomethine ylides, generated via the decarboxylative condensation of 1,3-thiazolidine-4-carboxylic acids with aldehydes, afforded 5,7a-dihydro-1H,3H-pyrrolo[1,2-c]thiazole derivatives. 2-Substituted-1,3-thiazolidine-4-carboxylic acids led to the stereoselective formation of 5,7a-dihydro-1H,3H-pyrrolo[1,2-c]thiazoles. Quantum-chemistry calculations were carried out allowing the rationalization of the observed stereoselective formation of the anti-dipole. Graphical abstractpor
dc.language.isoengpor
dc.publisherElsevierpor
dc.rightsopenAccesspor
dc.titleIntermolecular cycloaddition of nonstabilized azomethine ylides generated from 1,3-thiazolidine-4-carboxylic acids: synthesis of 5,7a-dihydro-1H,3H-pyrrolo[1,2-c]thiazolespor
dc.typearticlepor
degois.publication.firstPage9861por
degois.publication.lastPage9871por
degois.publication.titleTetrahedronpor
dc.peerreviewedYespor
dc.identifier.doi10.1016/j.tet.2006.08.029-
degois.publication.volume62por
uc.controloAutoridadeSim-
item.grantfulltextopen-
item.languageiso639-1en-
item.fulltextCom Texto completo-
crisitem.author.deptFaculdade de Ciências e Tecnologia, Universidade de Coimbra-
crisitem.author.deptFaculdade de Farmácia, Universidade de Coimbra-
crisitem.author.parentdeptUniversidade de Coimbra-
crisitem.author.researchunitCoimbra Chemistry Center-
crisitem.author.researchunitCoimbra Chemistry Center-
crisitem.author.orcid0000-0002-8264-6854-
crisitem.author.orcid0000-0003-3256-4954-
Appears in Collections:FCTUC Química - Artigos em Revistas Internacionais
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